原帖由： Alimpan ,
Well, the simplest way is that you go to the Videos app, then slide to the left on the video you want to delete (same works with Mail, and few other apps like iBooks) and a delete button (red colored) slides in to the right. You click the button, and your video gets deleted. Then in future, if you don't want to sync that video again, 1> Delete from your iTunes library OR 2> Uncheck 'Sync all videos' under the Videos tab in iTunes. Then it will not sync the video further, and you are left in peace to sync the desired videos.